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#! Ne atom RASCI/cc-pVQZ 
#! Example of split-virtual CISD[TQ] from Sherrill and Schaefer,
#! J. Phys. Chem. XXX
#! This uses a "primary" virtual space 3s3p (RAS 2), a "secondary" virtual
#! space 3d4s4p4d4f (RAS 3), and a "tertiary" virtual space consisting
#! of the remaining virtuals.  First, an initial CISD computation is run
#! to get the natural orbitals; this allows a meaningful partitioning of
#! the virtual orbitals into groups of different importance.  Next, the
#! RASCI is run.  The split-virtual CISD[TQ] takes all singles and doubles,
#! and all triples and quadruples with no more than 2 electrons in the
#! secondary virtual subspace (RAS 3).  If any electrons are present in
#! the tertiary virtual subspace (RAS 4), then that excitation is only allowed
#! if it is a single or double.
#

memory 250 mb

# First, get the natural orbitals

molecule ne {
  Ne
}

set globals {
  wfn detci
  basis cc-pVQZ
  d_convergence 10
# docc            [2, 0, 0, 0, 0, 1, 1, 1]
  frozen_docc     [1, 0, 0, 0, 0, 0, 0, 0]
  ex_level 2
}

set detci {
  nat_orbs_write true
}

set transqt2 {
  delete_tei false
}

psioh = psi4.IOManager.shared_object()
psioh.set_specific_retention(32, True)
psioh.set_specific_retention(33, True)
psioh.set_specific_retention(35, True)

thisenergy = energy('detci')


clean()

# !Warning: DGAS intentionally broke the second half here.

## Now, run the RASCI
#
#set globals {
#  wfn detci
#  d_convergence 10
#  docc            [2, 0, 0, 0, 0, 1, 1, 1]
#  frozen_docc     [1, 0, 0, 0, 0, 0, 0, 0]
#  ras1            [1, 0, 0, 0, 0, 1, 1, 1]
#  ras2            [1, 0, 0, 0, 0, 1, 1, 1]
#  ras3            [5, 2, 2, 2, 1, 3, 3, 3]
#  ex_level 2
#  val_ex_level 2
#}
#
#set detci {
#  maxiter 25
#  nat_orbs_write false
#
#  # This keyword is at the heart of the "split-virtual" CISD[TQ].
#  # If electrons are in RAS 4, do not allow the excitation to go beyond
#  # that specified by ex_level (here, only singles & doubles allowed if
#  # RAS 4 is populated)
#  mixed4 false
#  
#  # this will just reduce the number of strings generated in the
#  # computation; because of the mixed4=false specification above, not
#  # all of the strings normally allowed by the RAS will actually be needed
#  # in this computation
#  r4s true
#}
#
#thisenergy = energy('detci',bypass_scf='True')
#